Abstract:
Effect of Co, Ru and Cu substitution at B and B' sites on the magnetic and transport properties of LaSrCoRuO(6) have been investigated. All the doped compositions crystallize in the monoclinic structure in the space group P2(1)/n indicating a double perovskite structure. While the magnetization and conductivity increase in Co and Ru doped compounds, antiferromagnetism is seen to strengthen in the Cu doped samples. These results are explained on the basis of a competition between linear Co-O-Ru-O-Co and perpendicular Co-O-O-Co antiferromagnetic interactions and due to formation of Ru-O-Ru ferromagnetic networks.